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Angle-Resolved

Overview

In the angle-resolved cathodoluminescence (ARCL) mode, the direction in which a photon is emitted is determined. An objective lens or, more commonly, a collection mirror projects an image of the emitted light onto a pixelated detector, e.g., a camera. When an appropriate optical system is used, each pixel in the captured image corresponds to a unique emission direction from the specimen. The raw image is typically transformed into polar coordinates for display and interpretation.

 

The result of an angle-resolved measurement contains no wavelength or polarization information unless additional dispersion filtering is used (e.g., wavelength- and angle-resolved mode).

 

Angle-filtered information may be captured using an iris or a pinhole to select a specific (range of) angle(s). However, this particular acquisition mode's low resolution and highly serial nature have limited its usefulness.

“Schematic diagram showing angle‑resolved cathodoluminescence measurement setup.”
Sometimes referred to as Fourier imaging or momentum spectroscopy.
Angle‑resolved cathodoluminescence image showing directional emission patterns.
  

Data collection

Emission pattern or angle-resolved emission pattern

The emission pattern is a plot of the direction in which photons are emitted from a specimen. It is typically presented in polar coordinates, where the emission direction is described by the azimuthal and zenith angles. A single emission pattern may be captured from a point or region of the sample exposed to the electron beam of the electron microscope.

Angle‑resolved cathodoluminescence image showing directional emission pattern
Plots the emission pattern or angle-resolved emission pattern

Emission pattern image or angle-resolved spectrum image

The electron beam is scanned across the specimen surface, and an emission pattern is recorded at each location, creating a hyperspectral (4D) data construct.

“Angle‑resolved cathodoluminescence image showing directional emission pattern.”
Records an emission pattern image or angle-resolved spectrum image

Applications

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Uses

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